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Beilstein J. Org. Chem. 2015, 11, 1068–1078, doi:10.3762/bjoc.11.120
Graphical Abstract
Figure 1: Depictions of 9,10-bis(1,3-dithiol-2-ylidene)-9,10-dihydroanthracene (exTTF) in the (a) neutral for...
Scheme 1: Synthetic route to the target exTTF-based molecular wire 5.
Figure 2: Cyclic voltammograms of compound 5 and pristine exTTF (at concentrations of approximately 0.2 mM) u...
Figure 3: 2D histograms resulting from break junction experiments on an unmodified gold sample (a), OPE3-dith...
Figure 4: 2D histograms corresponding to compound 5 after exposing a gold substrate to the solution of the co...
Figure 5: 2D histograms corresponding to compound 5 after exposing a gold substrate to a solution of the comp...
Figure 6: a) Examples of individual G(z) traces showing clear conductance plateaus. b–e) 2D histograms corres...
Figure 7: Frontier orbitals of compound 5 in the gas phase.
Figure 8: Top a) and hollow b) binding geometries of 5 to a gold cluster in metal–molecule–metal junctions.
Figure 9: Transmission as a function of energy for the top and hollow binding geometries.